The enhanced sensing performance of ZnO-based photodetector by Mg doping

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Eka Nurfani, Lukman Nulhakim, Dwi Maulidia Muhammad, Monna Rozana, Widi Astuti

2024 Optical Materials Vol. 148 Article Cited by 27 Quartile

Abstract

In this paper, we study the effect of Mg on the structural, optical, and electrical properties of a ZnO-based photodetector. The sample was prepared by making a ZnO seed layer via spray pyrolysis. Then, the Mg-doped ZnO (MZO) nanorod was deposited on the seed layer via a hydrothermal technique with Mg concentrations of 0 wt% (ZnO), 1 wt% (MZ1), 3 wt% (MZ3), and 5 wt% (MZ5). From X-ray diffraction measurement, all samples show a hexagonal wurtzite structure. The nanorod formation of all samples was confirmed by scanning electron microscope images. Higher Mg dopant increases nanorod size from 872 ± 8 nm (pure ZnO) to 1764 ± 85 nm (5 % Mg). UV–Vis spectroscopy analysis shows that the bandgap generally increases with increased Mg content. Mg doping increases not only photoconductivity but also UV sensitivity by about 6 (ZnO), 46 (MZ1), 69 (MZ3), and 321 (MZ5). Responsivity increases linearly from 0.13 (ZnO) to 73.34 A/W (MZ5), and detectivity also increases linearly from 8.29×108 (ZnO) to 1.56×1011 Jones (MZ5). This study is essential to realize photodetector devices with low-cost fabrication techniques. © 2024 Elsevier B.V.

Affiliations

Department of Materials Engineering, Institut Teknologi Sumatera, Lampung, 35365, Indonesia; Department of Engineering Physics, Institut Teknologi Sumatera, Lampung, 35365, Indonesia; Research Center for Environmental and Clean Technology, National Research and Innovation Agency, Bandung, 40135, Indonesia; Research Center of Mining Technology, National Research and Innovation Agency of Indonesia, Lampung, 35361, Indonesia